Not all types of secondary organic aerosol mix: two phases observed when mixing different secondary organic aerosol types Atmospheric Chemistry and Physics DOI 10.5194/acp-22-13783-2022 11 January 2023 The number of condensed phases in mixtures of different secondary organic aerosol (SOA) types determines their impact on air quality and climate. Here we observe the number of phases in individual particles that contain mixtures of two different types of SOA. We find that SOA mixtures can form one- or two-phase particles, depending on the difference in the average oxygen-to-carbon (O/C) ratios of the two SOA types that are internally mixed within individual particles. Read more
Dynamics of the Great Oxidation Event from a 3D photochemical–climate model Climate of the Past DOI 10.5194/cp-18-2421-2022 9 January 2023 In the context of understanding the 3D photochemical effect on the Earth’s oxygenation that happened around 2.4 Ga, we developed a 3D photochemical–climate model to investigate the possible impact of atmospheric circulation and the coupling between the climate and the dynamics of oxidation. We show that the diurnal, seasonal and transport variations do not bring significant changes compared to 1D models. Nevertheless, we highlight a temperature dependence for atmospheric photochemical losses. Read more
Is it possible to estimate aerosol optical depth from historic colour paintings? Climate of the Past DOI 10.5194/cp-18-2345-2022 6 January 2023 This study investigates the possibility of inferring information on aerosol optical depth from photographs of historic paintings. The idea – which has been applied in previous studies – is very interesting because it would provide an archive of the atmospheric aerosol loading covering many centuries. We show that twilight colours depend not only on the aerosol optical thickness, but also on several other parameters, making a quantitative estimate of aerosol optical depth very difficult. Read more
Exceptional freshening and cooling in the eastern subpolar North Atlantic caused by reduced Labrador Sea surface heat loss Ocean Science DOI 10.5194/os-18-1507-2022 4 January 2023 Observations of the eastern subpolar North Atlantic in the 2010s show exceptional freshening and cooling of the upper ocean, peaking in 2016 with the lowest salinities recorded for 120 years. Using results from a high-resolution ocean model, supported by observations, we propose that the leading cause is reduced surface cooling over the preceding decade in the Labrador Sea, leading to increased outflow of less dense water and so to freshening and cooling of the eastern subpolar North Atlantic. Read more
Opinion: Coordinated development of emission inventories for climate forcers and air pollutants Atmospheric Chemistry and Physics DOI 10.5194/acp-22-13201-2022 2 January 2023 Emissions into the atmosphere of greenhouse gases (GHGs) and air pollutants, quantified in emission inventories, impact human health, ecosystems, and the climate. We review how air pollutant and GHG inventory activities have historically been structured and their different uses and requirements. We discuss the benefits of increasing coordination between air pollutant and GHG inventory development efforts, but also caution that there are differences in appropriate methodologies and applications. Read more
High-resolution drought simulations and comparison to soil moisture observations in Germany Hydrology and Earth System Sciences DOI 10.5194/hess-26-5137-2022 30 December 2022 In this paper, we deliver an evaluation of the second generation operational German drought monitor (www.ufz.de/duerremonitor) with a state-of-the-art compilation of observed soil moisture data from 40 locations and four different measurement methods in Germany. We show that the expressed stakeholder needs for higher resolution drought information at the one-kilometer scale can be met and that the agreement of simulated and observed soil moisture dynamics can be moderately improved. Read more
Early life stages of a Mediterranean coral are vulnerable to ocean warming and acidification Biogeosciences DOI 10.5194/bg-19-4767-2022 28 December 2022 For the first time, our study highlights the synergistic effects of a 9-month warming and acidification combined stress on the early life stages of a Mediterranean azooxanthellate coral, Astroides calycularis. Our results predict a decrease in dispersion, settlement, post-settlement linear extension, budding and survival under future global change and that larvae and recruits of A. calycularis are stages of interest for this Mediterranean coral resistance, resilience and conservation. Read more
The potential for using video games to teach geoscience: learning about the geology and geomorphology of Hokkaido (Japan) from playing Pokémon Legends: Arceus Geoscience Communication DOI 10.5194/gc-5-325-2022 26 December 2022 The fictional landscape of Hisui from Pokémon Legends: Arceus is inspired by the real-world island of Hokkaido, Japan. This paper illustrates how the game can be used to explore geological concepts including volcanology, economic geology, and hazard mitigation, by comparing in-game features to their real-world counterparts on Hokkaido. Applications from this study include increasing geoscientific interest and facilitating the self-learning or formal teaching of geoscience worldwide. Read more
Improving hydrologic models for predictions and process understanding using neural ODEs Hydrology and Earth System Sciences DOI 10.5194/hess-26-5085-2022 23 December 2022 Neural ODEs fuse physics-based models with deep learning: neural networks substitute terms in differential equations that represent the mechanistic structure of the system. The approach combines the flexibility of machine learning with physical constraints for inter- and extrapolation. We demonstrate that neural ODE models achieve state-of-the-art predictive performance while keeping full interpretability of model states and processes in hydrologic modelling over multiple catchments. Read more
The Antarctic contribution to 21st-century sea-level rise predicted by the UK Earth System Model with an interactive ice sheet The Cryosphere DOI 10.5194/tc-16-4053-2022 21 December 2022 The UK Earth System Model is the first to fully include interactions of the atmosphere and ocean with the Antarctic Ice Sheet. Under the low-greenhouse-gas SSP1–1.9 (Shared Socioeconomic Pathway) scenario, the ice sheet remains stable over the 21st century. Under the strong-greenhouse-gas SSP5–8.5 scenario, the model predicts strong increases in melting of large ice shelves and snow accumulation on the surface. The dominance of accumulation leads to a sea level fall at the end of the century. Read more